Modeling of a non-equilibrium dispersed phase and its fragmentation
In the context of the sustainable use of nuclear energy to produce carbon-free electricity, fourth-generation reactors, also known as "fast neutron" reactors, are necessary to close the fuel cycle.
This thesis falls within the framework of safety studies associated with such sodium-cooled reactors, and more particularly the hypothetical situation of a molten core relocating by gravity towards the core catcher at the bottom of the reactor vessel. A jet of corium (mixture of molten fuel and structural elements of the core) then interacts violently with the coolant, inducing, among other things, the fragmentation of the corium jet into droplets coupled with film boiling of the coolant. Characteristics of the resulting dispersed phase of corium and its fragmentation are crucial for studying the risk of runaway and steam explosion.
The aim of this thesis is to model a dispersed phase and its fragmentation in a surrounding fluid, using an approach that is both efficient and able to account to the scale variations and thermal imbalances between the droplets and the carrier phase. The method considered to meet these objectives is the method of moments, which derives from a kinetic model. It requires adequate closure and numerical schemes that satisfy non-standard constraints, while offering, in return, a crucial cost/accuracy compromise in the context studied. The advancements will be a priori implemented in the CFD software SCONE, built on the CEA's open-source TRUST platform.
The main work location will be based at the LMAG (Laboratory of Severe Accidents Modeling) at the IRESNE Institute of CEA Cadarache. Part of the work will also be carried out at the EM2C Laboratory (Molecular and Macroscopic Energetics, Combustion) – CNRS/CentraleSupélec in Paris.
The future PhD will work in a scientific dynamic environment and will acquire skills enabling to aspire to academic and industrial R&D positions.
Keywords : Dispersed Phase, Fragmentation, Kinetic, Method of Moments, Multiphase, Numerical methods, Severe Accidents.
Design artificial intelligence tools for tracking Fission Product release out of nuclear fuel
The Laboratory for the Analysis of Radionuclide Migration (LAMIR), part of the Institute for Research on Nuclear Systems (IRESNE) at CEA Cadarache, has developed a set of advanced measurement methods to characterize the release of fission products from nuclear fuel during thermal transients. Among these innovative tools is an operando in situ imaging system that enables real-time observation of these phenomena. The large amount of data generated by these experiments requires dedicated digital processing techniques that account for both the specificities of nuclear instrumentation and the underlying physical mechanisms.
The goal of this PhD project is to develop an optimized data processing approach based on state-of-the-art Artificial Intelligence (AI) methods.
In the first phase, the focus will be on processing thermal sequence images to detect and analyze material movements, aiming to identify an optimal image-processing strategy defined by rigorous quantitative criteria.
In the second phase, the methodology will be extended to all experimental data collected during a thermal sequence. The long-term objective is to create a real-time diagnostic tool capable of supporting experiment monitoring and interpretation.
This PhD will be carried out within a collaborative framework between LAMIR, which has recognized expertise in nuclear fuel behavior analysis and imaging, and the Institut Fresnel in Marseille, known for its strong background in image analysis and artificial intelligence.
The candidate will benefit from a multidisciplinary and stimulating research environment, with opportunities to present and publish their work at national and international conferences and in peer-reviewed journals.
Development of manganese-doped uranium oxide fuel: sintering mechanisms and microstructural changes
This PhD project focuses on developing nuclear fuels with improved properties through the addition of a dopant, for use in pressurized water reactors.
In nuclear reactors, the fuel consists of uranium dioxide (UO2) pellets stacked inside zirconium alloy cladding. These pellets, in contact with the cladding, must withstand extreme conditions of temperature and pressure. One of the challenges is to limit chemical interactions that may occur during the migration of fission products from the center to the periphery of the pellet and with the cladding. A notable example of such a phenomenon is the stress corrosion assisted by iodine, which can occur during accidental transients.
One strategy is to dope the UO2 ceramic with a metal oxide in order to control the material’s microstructure and also to modify its thermochemical behavior, thereby limiting both the mobility and corrosive nature of fission gases. Among the possible dopants, manganese oxide (MnO) represents a promising option and a potential alternative to chromium oxide (Cr2O3), which is currently a mature solution for the industry.
This PhD will explore the role of manganese in the sintering of UO2, particularly the microstructure and final properties of the fuel. The work will take place at the CEA Cadarache center, within the Institute for research on nuclear systems for low-carbon energy production (IRESNE).
During these three years, you will be hosted in the Laboratory for the study of uranium-based fuels (LCU) within the fuel study department (DEC), in close connection with the Laboratory for fuel behavior modeling (LM2C).
This research, combining experimentation and modeling, will be structured around three main topics:
• Study of the influence of manufacturing conditions on the microstructure of Mn-doped UO2,
• Investigation of the impact of doping on defect formation in UO2 and the associated properties,
• the contribution to the thermodynamic modelling of the system, based on experimental tests.
During this PhD, you will gain solid experience in the fabrication and advanced characterization of innovative materials, particularly in the field of ceramics for the nuclear industry. Your work could lead to publications, patents, and participation in national and international conferences.
You will also acquire numerous technical skills applicable across various research and industrial fields, including energy, microelectronics, chemical and pharmaceutical industries.
Atomistic investigation of the thermophysical properties of metallic nuclear fuel UMo
Uranium – molybdenum alloys UMo present excellent thermal properties and a good uranium density. For those reasons, they are considered as nuclear fuel candidates for research reactors. It is therefore crucial for the CEA to deploy new computational methodologies in order to investigate the evolution of their thermo-physical properties under irradiation conditions.
This project is centered on the application of atomistic methods in order to investigate the stability and diffusion of intra-granular xenon clusters within the metallic nuclear fuel UMo.
The first step of your work will involve continuing the development of atomic-scale computational models for UMo, as initiated within the host laboratory. These models use machine learning methods to develop interatomic potentials and will be validated by comparison with existing experimental data for this material. They will then be used to assess the temperature-dependent evolution and the impact of defect accumulation (both point and extended defects) on several thermophysical properties critical to fuel modeling, such as elastic properties, density, thermal expansion, as well as thermal properties like specific heat and thermal conductivity. In collaboration with other researchers in the department, you will format these results for integration into the Scientific Computing Tools used to simulate the behavior of nuclear fuels.
In a second phase, you will be responsible for extending the validity of your models to account for the formation of fission gases such as xenon within UMo single crystals. This will enable you to simulate the stability of xenon clusters in UMo crystals. These calculations, performed using classical molecular dynamics methods, will be systematically compared with experimental observations obtained via transmission electron microscopy.
The results obtained during the various stages of this project will be completely innovative and will be the subject of scientific publications as well as presentations at international scientific conferences. Besides, this work will enable you to complement your training by acquiring skills applicable to many areas of materials science, including ab initio calculations, machine learning-based interatomic potential fitting, classical molecular dynamics, use of CEA supercomputers, and key concepts in statistical physics and condensed matter physics—fields in which the supervising team members are recognized experts.
You will join the Fuel Behavior Modeling Laboratory at the Research Institute for Nuclear Systems for Low-Carbon Energy Production (IRESNE, CEA Cadarache), a dynamic research team where you will have regular opportunities to interact with fellow PhD students and researchers. This environment also provides extensive opportunities for national and international collaboration, including with:
• Developers and users of the MAIA fuel performance code (dedicated to research reactor fuel studies),
• Experimental researchers from the Nuclear Fuel Studies Department,
• Teams from other CEA centers (Saclay, CEA/DAM),
• International partners.
This rich and multidisciplinary context will enable you to fully engage with the scientific community focused on nuclear materials science.
[1] Dubois, E. T., Tranchida, J., Bouchet, J., & Maillet, J. B. (2024). Atomistic simulations of nuclear fuel UO2 with machine learning interatomic potentials. Physical Review Materials, 8(2), 025402.
[2] Chaney, D., Castellano, A., Bosak, A., Bouchet, J., Bottin, F., Dorado, B., ... & Lander, G. H. (2021). Tuneable correlated disorder in alloys. Physical Review Materials, 5(3), 035004.
UO2 Powders: Morphological Characterization of Aggregates and Study of Their Interactions Using a Combined Experimental and numerical Approach
This PhD thesis is part of the optimization of nuclear fuel fabrication processes, which rely on the powder metallurgy of uranium dioxide (UO2) and plutonium dioxide (PuO2). These powders exhibit a hierarchical microstructure composed of crystallites forming rigid aggregates, themselves agglomerated into larger structures. The morphology and interactions between aggregates play a key role in the macroscopic behavior of the powders—particularly their flowability, compressibility, and agglomeration capacity—and directly influence the quality of the fuel pellets obtained after pressing and sintering. However, the experimental characterization of these aggregates remains complex and does not yet allow for the establishment of a predictive link between synthesis processes and morphological properties.
The objective of this thesis is to combine experimental and numerical approaches to achieve a detailed characterization of the aggregates in a reference powder. Experimentally, techniques such as Scanning Electron Microscopy (SEM), specific surface area measurement (BET), and laser granulometry will be used to determine particle size, roughness, and size distribution. In parallel, numerical simulations based on the Discrete Element Method (DEM) will be employed to construct a granular digital twin consistent with the experimentally measured properties. This digital twin will allow the reconstruction of the internal structure of the aggregates, the evaluation of interparticle adhesion forces, and the analysis of agglomeration and densification phenomena under controlled conditions.
The PhD will take place at CEA Cadarache within the Institute for Research on Nuclear Systems for Low-Carbon Energy Production (IRESNE). The student will be assigned to the PLEIADES Fuel Development Laboratory (LDOP), which specializes in simulating nuclear fuel behavior (from fabrication to in-reactor performance) and in multi-scale numerical methods. The work will be carried out in collaboration with the CNRS/LMGC in Montpellier, internationally recognized for its research on granular materials, and with the Uranium Fuel Laboratory (LCU – CEA Cadarache), which has extensive experience in the experimental characterization of uranium powders.
The PhD candidate is expected to demonstrate strong skills in numerical simulation and in the physical analysis of results. He will share its results through publications and conference presentations and will have the opportunity to learn or further develop various experimental and numerical techniques that can be applied in other contexts.In particular, the issues related to the physics of granular media — which constitute the core of this PhD — are of significant industrial relevance and are common to many other sectors handling powders, such as pharmaceuticals, agri-food, and powder metallurgy.
[Hebrard2004] S.Hebrard, Etude des mécanismes d’évolution morphologique de la structure des poudres d’UO2 en voie sèche, thèse de doctorat, CEA-LSG2M-COGEMA), 2004.
[Pizette2010] P. Pizette, C.L. Martin a, G. Delette, P. Sornay, F. Sans, Compaction of aggregated ceramic powders: From contact laws to fracture and yield surfaces, Powder Technology, 198, 240-250, 2010.
[Tran2025] T.-D. Tran , S. Nezamabadi , J.-P. Bayle, L. Amarsid, F. Radjai , Effect of interlocking on the compressive strength of agglomerates composed of cohesive nonconvex particles, Advanced Powder Technology 36, 2025.
Micromechanical Modeling of the Behavior of Polycristals with Imperfect Interfaces: Application to Irradiated UO2 Fuel
This thesis aims to analyze the thermomechanical properties of UO2 fuel used in pressurized water reactors (PWRs), accounting for the effects of microscopic defects. It focuses particularly on intergranular decohesion phenomena observed at various stages of fuel evolution, notably prior to crack initiation and propagation. The objective of this thesis is to clarify the impact of decohesion on both the local and effective properties of UO2 during irradiation. To this end, intergranular decohesion is modeled at the local scale by means of imperfect interface models, which ensure traction continuity while allowing for a displacement jump at grain boundaries. This modeling approach enables the development of homogenization models incorporating innovative theoretical and numerical advances, capable of capturing the behavior of the fuel at very high temperatures, under off-normal and accidental conditions. This work will be conducted at CEA Cadarache,in the Institute for Research on Nuclear Systems for Low-Carbon Energy Production (IRESNE), in close collaboration with national and international research teams. The tools developed will contribute to improving our understanding of the fuel's properties and to enhancing the accuracy and reliability of existing models, particularly those implemented in the PLEIADES simulation platform developed by the CEA in collaboration with French nuclear industry partners.
Nuclear fuel fragmentation under thermal gradient of fuel during laser heating: correlation, numerical simulation and and adaptation of the experimental setup.
The aim of this thesis is to simulate the cracking of nuclear fuel, which consists of a brittle ceramic material, uranium dioxide, during laser heating experiments. The objective is to compare the numerical results with experimental data through image correlation. This comparison will make it possible to optimize the experimental setup, improve the quality of the experimental results, and move toward a quantitative validation of the gradient damage models used in the simulations.
The starting point of this work is a campaign of uranium dioxide pellet fragmentation by laser heating, carried out as part of the PhD of Hugo Fuentes [1] in one of the experimental laboratories of the Institute for Research on Nuclear Energy Systems for Low-Carbon Energy Production (IRESNE) at CEA Cadarache (DEC/SA3E/LAMIR). This heating technique reproduces temperature gradients representative of reactor conditions. For each test, films showing the evolution of cracks and surface temperature changes in the pellet are available.
These films will be analyzed by digital image correlation (DIC) [3] using an in-house software tool to determine optimal boundary conditions for the numerical simulations and extract relevant data for model validation. The experiments will then be modeled using gradient damage models developed in the PhD theses of David Siedel and Pedro Nava Soto [2]. Based on the results obtained, the PhD candidate will be able to optimize and/or adapt the setup to study other operating conditions and conduct a new experimental campaign.
The PhD student will work in close collaboration between a simulation laboratory and an experimental laboratory within the IRESNE Institute at CEA Cadarache. The proposed work is open-ended and may be promoted through participation in national or international conferences and the publication of scientific articles in high-impact journals.
References
[1] Fuentes, Hugo, Doualle, Thomas, Colin, Christian, Socié, Adrien, Helfer, Thomas, Gallais, Laurent, and Lebon, Frédéric. Numerical and experimental simulation of nuclear fuel fragmentation via laser heating of ceramics. In: Proceedings of Top Fuel 2024, Grenoble, 29 September 2024.
[2] Nava Soto, Pedro, Fandeur, Olivier, Siedel, David, Helfer, Thomas, and Besson, Jacques. Description of thermal shocks using micromorphic damage gradient models. European Solid Mechanics Conference, Lyon, 2025.
[3] Castelier Etienne, Rohmer E., Martin E., Humez B. Utilisation de la dimension temporelle pour ameliorer la
correlation d'images. 20 eme Congres Francais de Mecanique, 2011.
Fluid-structure coupling with Lattice-Boltzmann approach for the analysis of fast transient dynamics in the context of hydrogen risk
With a view to preparing for the future in the field of high-fidelity, high-performance simulation, the CEA is working with its academic and industrial partners to explore the potential of fluid-structure couplings involving Lattice Boltzmann Methods (LBM). The coupling is part of an open-source standard promoted by the CEA, and promising first steps have been taken for compressible flows interacting with structures undergoing large displacements and rupture. Significant obstacles remain to be overcome, particularly for more complex fluid representations that are representative of industrial needs, especially for the safety of carbon-free energy devices such as batteries and nuclear reactors.
This doctoral work therefore focuses on extending the available basic building blocks to the case of flame propagation in hydrogen/air mixtures, in deflagration and detonation regimes with possible transition between the two, and in interaction with flexible structures undergoing finite displacement. This presupposes, in particular, the consideration of compressible flows with high Mach numbers significantly exceeding those used to date, requiring an in-depth reanalysis of coupling schemes and fluid-structure interaction techniques.
The thesis will be part of a collaboration between the IRESNE Institute (CEA Cadarache) and the M2P2 laboratory (AMU). The work will be mostly localized at M2P2 with a close methodological supervision from IRESNE, especially in the field of coupling techniques.
DEM-LBM Coupling for simulating the ejection of immersed granular media in compressible Fluid under High Pressure Gradients
In Pressurized Water Reactors (PWRs), the fuel consists of uranium oxide (UO2) pellets stacked in metallic cladding. During a Loss of Coolant Accident (LOCA) scenario, the rapid temperature increase can cause deformation and sometimes rupture of these claddings. This phenomenon can potentially lead to the ejection of fuel fragments into the primary circuit. This phenomenon is known as FFRD (Fuel Fragmentation, Relocation, and Dispersal). Since the cladding is the first safety barrier, it is crucial to evaluate the amount of dispersed fuel. Experimental studies have shown that the size, shape of the fragments, shape of the breach, and internal pressure significantly influence the ejection. However, the speed of the initial depressurization phase makes direct measurements difficult. Numerical approaches, particularly through fluid-grain coupling (LBM-DEM), offer a promising alternative. The IRESNE Institute at CEA Cadarache, through the PLEIADES software platform, is developing these tools to model the behavior of fragments. However, the compressibility of the gas needs to be integrated to accurately reproduce the initial depressurization. In this context, the laboratory M2P2 of the CNRS, a specialist in modeling compressible flows with the LBM method and developer of the ProLB software, brings its expertise to integrate this effect. The thesis therefore aims to design and improve a compressible model in the LBM-DEM coupling, to conduct a parametric study, and to develop a 3D HPC demonstrator capable of leveraging modern supercomputers.
This CEA thesis will be conducted in close collaboration between the Fuels Research Department (DEC) of the IRESNE Institute at CEA Cadarache and the laboratory M2P2 (CNRS). You will be primarily located at M2P2 but will make regular visits to CEA within the Fuel Simulation Laboratory, to which you will be affiliated. The approaches developed in this thesis ensure a high scientific level with numerous potential industrial applications both within and outside the nuclear field.
Shape optimization for innovation in nuclear fuels
Nuclear industry is currently developping enhanced Accident Tolerant Fuels" (ATF) [1]. These fuels feature enhanced physical properties; in particular, thanks to the addition of thermal conductors inside the fuel, they tend to be colder in standard as well as in accident conditions.
This thesis aims at developping numerical strategies (that will be programmed into a semi-industrial code) in order to propose new "shapes" of fuels (by "shape", we mean internal structures or microstructures), and to optimze already existing concepts. It will take advantage of recent numerical and mathematical techniques related to the so-called "shape optimization" [2]. Based on the previous work [3], more and more complex physical phenomena will be taken into account : first, thermal conductivity and mechanical behaviour in standard conditions, then gaz diffusion... Discussion with experts and modelization will be necessay in order to reformulate these physical behaviours into forms amenable to numerical simulation.
This thesis will take place at the CEA center of Cadarache in the fuel research department, in a laboratory devoted to modelling and numerical methods. The latter is affiliated to the Institute IRESNE for the research low-carbon energy production.
This project will be in collaboration with Nice University offering so an environment both academic and connected to application.
It also takes part in the PEPR DIADEM called Fast-in-Fuel, a national research project.
We search for excellent candidates with a solid background in scientific computing, analysis and numerical analysis of partial differential equations, as well as in optimization. Skills in physics (mechanics and thermics) will also be considered. The proposed subject aims at a concrete application at the intersection of various scientific fields, and it is largely exploratory. Hence, curiosity and creativity will also be highly appreciated.
[1] Review of accident tolerant fuel concepts with implications to severe accident progression and radiological releases, 2020.
[2] G. Allaire. Shape optimization by the homogenization method, volume 146 of Applied Mathematical Sciences. Springer-Verlag, New York, 2002.
[3] T. Devictor. PhD Manuscript, 2025 (in preparation)