Nuclear data is crucial for civil nuclear energy applications, being the bridge between the micoscopic properties of nuclei and the “macroscopic good values” needed for cycle and reactor physics studies. The laboratory of physics studies at CEA/IRESNE Cadarache is involved in the evaluation of these nuclear physics observables, in the framework of the JEFF Group and the Coordinated Research Project (CRP) of IAEA. The recent development of a new methodology for thermal neutrons induced fission product yield evaluation (fission product yields after prompt neutron emission) has improved the accuracy of the evaluations proposed for the JEFF-4.0 Library, together with their covariance matrix. To extend the assessments of fission yields induced by thermal neutrons to the fast neutron spectrum, it is necessary to develop a coupling of current evaluation tools with fission fragment yield models (before prompt neutron emission). This coupling is essential to extrapolate the actual studies on thermal fission of 235U and 239Pu to less experimentally known nuclei (241Pu, 241Am, 245Cm) or to study the incident neutron energy dependence of fission yields. One of the essential missing components is the description of the nuclear charge distribution (Z) as a function of the mass of the fission fragments and the incident neutron energy. These distributions are characterized by a key parameter: the charge polarization. This polarization reflects an excess (respectively deficiency) of proton in light (respectively heavy) fission fragments compared to the average charge density of the fissioning nucleus. If this quantity has been measured for the 235U(nth,f) reaction, it is incomplete for other neutron energies or other fissioning systems. The perspectives of this subject concern as much the impact of these new evaluations on the key quantities for electronuclear applications as well as the validation of the fission mechanisms described by microscopic fission models.

The ability of nuclear models to accurately predict the rich phenomenology emerging in nuclei (whether for fundamental purposes or nuclear data applications) is conditioned by the possibility to construct a systematically improvable theoretical framework, i.e. with controlled approximations and estimation of associated uncertainties and biases. This is the goal of so called ab initio methods, which rely on two steps:
1 - The construction of an inter-nucleon interaction in adequation with the underlying theory (quantum chromodynamics) and adjusted in small systems, following effective field theory paradigm.
2 - The resolution of nuclear many-body problem to a given accuracy (for structure or reactions observables). This provides predictions in all nuclei of interest and includes the uncertainty propagation stemming from the interaction model up to nuclear data predictions.

This PhD thesis mostly deals with Step 1. The goal of the thesis is to construct a family of ab initio interactions by developing a new adjustment procedure of the low energy constants (including the evaluation of covariances for sensitivity analysis). The adjustment will include structure data but also reaction observables in light systems. This will open the door to a new evaluation of p+n->d+gamma cross sections (which have large uncertainties despite their importance for neutronics applications) in the context of state-of-the-art effective fields theories.

The thesis will be done in collaboration between CEA/IRESNE (Cadarache) and IJCLab (Orsay), the PhD student will spend 18 months in each laboratories. Professional perspectives are academic research and R&D labs in nuclear physics.