Study of uranium-235 fission induced by neutrons from 0.5 to 40 MeV at NFS-SPIRAL2 using the FALSTAFF spectrometer and the FIFRELIN code
The presented project has two main objectives. The first one is the realization (building, calibration, data taking and data analysis) of a first experiment with the FALSTAFF detector in its configuration with two detection arms. In such a configuration, FALSTAFF will be able to detect in coincidence both fragments emitted by fast-neutron triggered fission reactions. These neutrons will be provided by the neutron beam of SPIRAL2-NFS in GANIL. The advantage of using direct kinematics is the ability to determine on an event-by-event basis the excitation energy of the fissioning nucleus by the measurement of the incident-neutron kinetic energy.
For this first experiment, we will have a uranium 235 target. 235U is the main source of fission neutrons in nuclear reactors and therefore at the heart of the system. Hence, the understanding of neutron-induced fission of 235U is essential and the rather exclusive data FALSTAFF will provide, with not only the identification of the fission fragments but also their kinematics will permit to reconstruct also the fissioning system. Such a measurmement in direct kinematics have never been done, to our knowledge, with the accuracy we are aiming at.
To perform this exepriment, we have improved and added detection capabilities to the FALSTAFF spectrometer, in particular with the financial support of the Région Normandie over the last two years. This experiment will be completed by a work to be done on a theoretical model developed by our collaborators of CEA-Cadarache. We will compare our detailled data with predictions of the model and have the model evolve, according to the laws of nuclear physics in order to obtain results from the model close to the data. Such a test of this model on as complete data as those we will obtain with FALSTAFF have never been done so far.
Stochastic Neutron Noise Estimation Using a Rare-Event Simulation Approach. Application to the Monitoring of Nuclear System Reactivity
This PhD project aims to develop an innovative method to characterize the reactivity of fissile systems by analyzing their stochastic fluctuations, known as zero-power neutron noise. In a subcritical fissile medium, neutrons originating from spontaneous fission can initiate short and random chain reactions, generating a fluctuating signal. This noise carries essential information on the distance of the system to criticality, a key parameter both for the safety of nuclear installations (prevention of criticality accidents) and for the detection of undeclared fissile materials (nuclear security and non-proliferation).
Existing theoretical approaches to infer system reactivity from neutron noise are limited to idealized situations and become unsuitable in realistic configurations, particularly when the system is strongly subcritical or when significant uncertainties exist regarding its geometry or composition (as in the case of the Fukushima Daiichi corium or spent fuel storage). Monte Carlo simulations then appear as a natural alternative, but current simulations rely on variance reduction techniques that fail to correctly preserve stochastic fluctuations.
This thesis proposes to address this scientific challenge by adapting a relatively recent variance reduction method known as Adaptive Multilevel Splitting (AMS), originally developed to efficiently sample rare events while preserving their statistical properties. The goal is to extend this method to neutron transport in multiplying media and to make it a tool capable of faithfully simulating the temporal correlations characteristic of neutron noise. Following the theoretical developments, the algorithm will be implemented in Geant4, compared to analytical benchmark solutions, and experimentally validated through in situ measurements (using neutron sources or research reactors). In the long term, this work may lead to direct applications in nuclear monitoring, safety diagnostics, and detector physics, while also opening perspectives in fundamental physics and medical physics.
Exotic shape of the nucleus: decay spectroscopy of neutron-deficient actinides with the detector SEASON
The question of the limit of stability of nuclei, both in terms of proton/neutron asymmetry and in terms of mass, is an important open question in modern nuclear physics. In the region of heavy nuclei, the neutron-deficient actinides present a great interest. Indeed, strong octupolar deformation, giving a pear shape to the nuclei, are predicted and have event been already observed in some isotopes. These deformations seem to play a key role for nuclear stability, for nuclear decay modes, and may also be related to physics beyond the standard model. The main goal oh this thesis will be to pursue the systematic study of these deformations by making use of the brand-new SEASON detector, whose first experiment will take place at the University of Jyväskylä (Finland) in February 2026. The thesis will focus on the analysis of data from the experimental campaign that will occur in summer 2026. Several experiments are foreseen, making use of different beam-target combinations to produce actinides by fusion-evaporation reaction. These actinides will then be sent inside SEASON to perform their decay spectroscopy. Depending on the plannings, another campaign could be scheduled at Jyväskylä in 2027. Finally, the return of the instrument in France to be set up at GANIL-Spiral2 (Caen) coupled to the S3 spectrometer will certainly take place this the thesis period.
The thesis can be co-directed by the university of Jyväskylä.
Monitoring criticality risk through neutron noise in degraded nuclear environments
Our team at CEA/Irfu is working with ASNR to study the possibility of using neutron noise measurements, i.e., stochastic variations in neutron flux, to estimate the reactivity of subcritical nuclear systems. The aim is to propose this technique for online measurement of the reactivity of the corium at Fukushima Daiichi during future decommissioning operations. The thesis work will focus on evaluating a solution based on Micromegas-type neutron detectors (nBLM detectors) developed by IRFU, which are adapted to the extreme gamma radiation expected in the vicinity of the Fukushima Daiichi corium. The student will participate in experiments at nuclear research facilities in Europe and the United States to test this technical solution and measure neutron noise for a wide range of reactivities. He/she will be responsible for analyzing the data and evaluating the various inversion methods used to estimate reactivity from neutron noise measurements.
Measurement of low lying dipole excitations using neutron inelastic scattering
The pygmy dipole resonance is a vibration mode observed in neutron-rich nuclei and which has initially been described as the oscillation of a neutron skin against a symmetric core in term of proton and neutron numbers. But experimental studies have revealed a more complex structure. Few years ago, we have proposed to take benefit of the high intensity neutron flux from SPIRAL2-NFS to study the pygmy resonance with an original approach: the neutron inelastic scattering. Following the success of the first experiment carried out in 2022, we propose to continue our program in a new region of the nuclear chart. The objective of the thesis is to study the pygmy dipole resonance in 88Sr by inelastic neutron scattering. The thesis will consist of: i) participation in the experiment, ii) data analysis, and iii) interpretation of the results in collaboration with theorists.
Development of the Micromegas CyMBaL Detector and study of gluon saturation for the future electron-ion collider
The future Electron-Ion Collider (EIC), to be constructed at Brookhaven National Laboratory (NY, USA) is a next-generation facility designed to explore the inner structure of protons and nuclei with unprecedented precision. It will explore how quarks and gluons generate the mass, spin, and structure of visible matter, and study the increase of gluon density at small Bjorken-x. To meet its ambitious physics goals, innovative detectors are being developed — including the Micromegas CyMBaL system, a gaseous tracker for the central region of the first EIC experimental apparatus ePIC.
This PhD project combines experimental detector R&D and physics simulations:
* Prototype characterization: build and test full-scale Micromegas detectors; measure efficiency, gain uniformity, and spatial resolution in laboratory and beam environments. Test and validate the prototypes with the new ASIC SALSA developed at CEA for gasesous detectors at ePIC.
* Detector simulations: integrate the CyMBaL geometry into the EIC framework and assess global tracking and performance requirements.
* Physics studies: simulate key processes sensitive to gluon saturation (e.g. final-state di-hadron correlations) to understand QCD at small-x and evaluate how detector performance influences physics sensitivity.
The PhD student will have opportunities to participate in the development of state-of-the-art gaseous detectors and to work within an international community of hadronic physicists on topics at the forefront of the field, with trips to Brookhaven National Laboratory (NY, USA) and opportunities for test-beam campaigns at accelerator facilities.
INVESTIGATION OF THE NUCLEAR TWO-PHOTON DECAY
The nuclear two-photon, or double-gamma decay is a rare decay mode in atomic nuclei whereby a nucleus in an excited state emits two gamma rays simultaneously. This second-order electromagnetic process, well known in atomic physics, has been little studied for the atomic nucleus due to the largely predominant first-order processes. Even-even nuclei with a first excited 0+ state are favorable cases to search for a double-gamma decay branch, since the emission of a single gamma ray is strictly forbidden for 0+ to 0+ transitions by angular momentum conservation. The double-gamma decay still remains a very small decay branch (<1E-4) competing with the dominant (first-order) decay modes of atomic internal-conversion electrons (ICE) or internal positron-electron (e+-e-) pair creation (IPC).
The thesis project has two distinct experimental parts: First, we store bare (fully-stripped) ions in their excited 0+ state in the heavy-ion storage ring (ESR) at the GSI facility to search for the double-gamma decay in several nuclides. For neutral atoms the excited 0+ state is a rather short-lived isomeric state with a lifetime of the order of a few tens to hundreds of nanoseconds. At relativistic energies available at GSI, however, all ions are fully stripped of their atomic electrons and decay by ICE emission is hence not possible. If the state of interest is located below the pair creation threshold the IPC process is not possible either. Consequently, bare nuclei are trapped in a long-lived isomeric state, which can only decay by double-gamma emission to the ground state. The decay of the isomers is identified by so-called time-resolved Schottky Mass Spectroscopy. This method allows to distinguish the isomer and the ground state by their (very slightly) different revolution time in the ESR, and to observe the disappearance of the isomer peak in the mass spectrum with a characteristic decay time. Successful experiment establishing the double-gamma decay in several nuclides (72Ge, 98Mo, 98Zr) were already performed and a new experiment to study the nuclide 194Pb has been accepted by the GSI Programme Committee and its realization is planned for 2027.
The second part concerns the direct observation of the emitted photons using gamma-ray spectroscopy. While the storage ring experiments allow to measure the partial lifetime for the double gamma decay, further information on the nuclear properties can be only be achieved by measuring the photon themselves. A test experiment has been performed to study its feasibility and the plans a more detailed study should be developed with the PhD project.
Contribution of artificial intelligence to the study of fission
Nuclear fission is an extreme process during which a heavy nucleus deforms until it reaches a point of no return leading to its separation into two fragments. The process goes with a significant release of energy, mainly as kinetic energy of the newly formed fragments, but also as excitation energy (about 15 MeV/fragment). In addition, the fragments are also produced with a high angular momentum. It is through the emission of neutrons and photons that fission fragments evacuate their energy and angular momentum. The ultimate experiment in fission would consist of identifying each fragment in mass and charge; measuring their kinetic energy; and characterize in energy and multiplicity the neutrons and photons they emit. This data set would make it possible to access the global energy of the fission process and to completely characterize the deexcitation of the fragments. Due to the significant complexity of such an exclusive measurement, this data set is always missing.
Our team is moving towards such measurement and this thesis work aims to explore the benefits that machine learning techniques can bring in this perspective.
The thesis will consist of taking advantage of all the experimentally accessible multi-correlated data in order to feed machine learning algorithms whose purpose will be to identify fission fragments and determine their properties.
The developed techniques will be applied to a first data set using a twin ionization chamber for the detection of fission fragments coupled to a set of neutron detectors. The data will be acquired at the beginning of the thesis.
In a second step, a more exploratory study will consist of applying the same techniques to data obtained during the thesis using a temporal projection chamber as a fission fragment detector. It will be a matter of demonstrating that the energy resolution is compatible with the study of fission.
Study of heavy nuclei: from the mass measurement to the spectroscopy of Americium nuclei and commissioning of the double Penning trap PIPERADE
The atomic nucleus is a complex system that continues to be actively studied more than a century after its discovery. Among the open questions, the question of the limits of existence of the nucleus remains central: what are the numbers of protons and neutrons that allow a bound nucleus to form? This question can be addressed using mass measurements that provide access to the binding energy of the nucleus, one of its most fundamental properties. The objective of this thesis is, on the one hand, to perform high-precision mass measurements of the isotopes 234-238Am (Z = 95) isotopes at the University of Jyväskylä, Finland (experiment planned in 2026), and, on the other hand, to participate in the installation and commissioning of the PIPERADE double Penning trap (PIèges de PEnning pour les RAdionucléides à DESIR) at GANIL in Caen.
The americium nuclei that will be studied in this thesis are at the boundary between two regions of particular interest: the octupole deformation region (pear-shaped nuclei) and the fission isomer region (meta-stable states of nuclei decaying by fission), and measuring their mass will provide a better understanding of the properties of these exotic nuclei.
PIPERADE is a device that can be used to perform high-precision mass measurements. Currently in the characterisation phase in Bordeaux, its installation at GANIL will enable the study of a wide range of exotic nuclei by measuring their mass. Currently undergoing characterisation in Bordeaux, its installation at GANIL (planned for 2027) will enable the study of a wide range of exotic nuclei by measuring their mass, but also by using separation techniques to purify the radioactive beams before sending them to other experimental devices.
STUDY OF THE NUCLEAR COLLECTIVE PROPERTIES OF 232TH WITH THE AGATA SPECTROMETER
The study of so-called ‘deformed’ atomic nuclei with a non-spherical charge distribution is essential for testing nuclear interactions and structural models. These deformed nuclei exhibit a very particular pattern of excited states, known as ‘rotational bands’. These bands can be constructed on states with different deformations or different intrinsic structures (shape coexistence). The subject of the thesis is the experimental study of the macroscopic and microscopic properties of the nucleus 232Th. This nuclide exhibits a wide variety of rotational bands that are thought to be due to vibrations of the nuclear surface known as quadrupole and octupole vibrations. In particular the latter have attracted a great deal of interest recently, as octupolar deformed nuclei can be used to determine nuclear electric dipole moments, a fundamental question in physics in general. In our particular case, the aim is to characterise for the first time the quadruplet of octupole bands expected in a strongly deformed nucleus. Furthermore, this nucleus is the only example with a rotational band built on a double quadrupole vibration.
We will study these various shapes using the powerful technique of Coulomb excitation, which is the most direct method for determining the shape of nuclei in their excited states. The experiment will be carried out using AGATA, a new-generation gamma spectrometer consisting of a large number of finely segmented germanium crystals, which can identify each point of interaction of a gamma ray inside the detector and then, using the innovative concept of ‘gamma-ray tracking’, reconstruct the energies of all the gamma rays emitted and their emission angles with unprecedented precision. A complementary experiment will be carried out at HIL Warsaw, which will enable better interpretation of the highly complex data provided by AGATA.