Until recently, CO2 capture technologies were developed separately from CO2 utilization technologies, even though coupling the CO2 desorption stage with the chemical transformation of CO2, which is generally exothermic, would yield significant energy savings.
The first coupled solutions have recently been proposed, but they are mainly at moderate temperatures (100-180°C) [1], or even recently close to 225°C [2].
The objective of this doctoral thesis is to study, both experimentally and theoretically, a coupled system in the 250-325°C temperature range that allows via Fischer-Tropsch-type catalytic hydrogenation the direct production of higher value-added products